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Simple scenario of integrated neutron-proton interaction

  • In this study, we investigate the patterns exhibited by integrated neutron-proton interactions (denoted as VNP) that exhibit systematic differences among particle-particle, hole-hole, hole-particle, and particle-hole cases. A simple formula of VNP is proposed to be in approximate linearity with NnNp. This formula yields regular patterns of VNP that are highly consistent with those previously extracted according to binding energies. The observed ordering of VNP, i.e., VNP of the particle-particle case is the largest, VNP of the hole-hole case is in-between, and VNP of the particle-hole and hole-particle cases is the smallest, is explained in terms of the dominant part of VNP originating from symmetry energy and refinement involving the shell correction in the mass formulas.
  • Neutron-proton interactions play the most important role in the evolution of the shell structure, collectivity, phase shape transitions, and deformation, as stressed by de Shalit [1] and Talmi [2] and later by Federman and Pittel [3, 4]. The neutron-proton interaction was simplified and parametrized as NpNn, i.e., the product of the valence proton number and valence neutron number, by Casten [5]. This is called the NpNn scheme in literature, or in a more semantic meaning, the valence correlation scheme [6, 7]. Zhang and collaborators [8], and later Fu et al. [9], empirically extracted integrated neutron-proton interactions (denoted as VNP) by using the experimental atomic masses, and a remarkable linearity between VNP and NpNn was shown for the case with 50<Z<82 and 50<N<82. Recently, it was demonstrated [10] that such integrated neutron-proton interactions exhibit systematic differences for the particle-particle, hole-hole, and particle-hole cases in the (50<Z<82 and 82<Z<126) major shells. This pattern is a reflection of the differences in the average neutron-proton interactions of those three cases, as pointed out earlier by Cakirli and Casten in Ref. [11]. For completeness, we mention Refs. [1218], in which neutron-proton interactions were also studied from other perspectives.

    The purpose of this paper is to provide a simple scenario for the above interesting pattern of integrated neutron-proton interactions. We show that these regularities essentially originate from nuclear symmetry energy, with a subtle effect from the shell correction. We also present a compact formula of VNP in terms of NnNp.

    The remainder of this paper is organized as follows. In Sec. II, we derive the formula of VNP based on the improved liquid-drop model with the shell correction [19]. In Sec. III, we discuss the contributions of the Wigner energy and the shell effect to the VNP, and in Sec. IV, we discuss the linear correlation between VNP and NpNn as well as the relative magnitudes of the particle-particle, hole-hole, particle-hole, and hole-particle cases. In Sec. V, we summarize this paper.

    In this section, we present the values of VNP extracted by using theoretical binding energies of the WS3 model [19] and compare these empirical results for VNP with those calculated via our simple formula of VNP derived from the liquid-drop model with the shell correction. We shall see remarkable consistency between VNP values obtained via these two approaches.

    Let us begin our discussion with the definition of VNP. According to Eqs. (4)–(5) of Ref. [9], the empirical integrated neutron-proton interaction is expressed as follows:

    VNP(Z,N)=14δpδn[S(Z,N)+S(Z0,N0)S(Z0,N)S(Z,N0)],

    (1)

    where δp (δn) is +1 if the valence protons (neutrons) are particle-like and 1 if the valence protons (neutrons) are hole-like, Z0 (N0) is the nearest magic number for protons (neutrons), and S(Z,N) is defined as

    S(Z,N)=B(Z+δp,N+δn)+B(Z+δp,N)+B(Z,N+δn)+B(Z,N),

    (2)

    where B represents the nuclear binding energy. For convenience, in this paper, we use the convention that the values of B are positive; with this convention, the values of VNP are positive.

    In Fig. 1, we plot such extracted VNP values versus NpNn from the improved Weizsäcker mass formula (WS3) [19] for numerous major shells: (28<Z<50, 28<N<50), (28<Z<50, 50<N<82), (50<Z<82, 50<N<82), and (50<Z<82, 82<N<126). These empirical neutron-proton interactions are plotted in panels (a-d), with blue color for the particle-particle case, red for the hole-hole case, green for the particle-hole case, and violet for the hole-particle case. One also sees that the extracted VNP values have a good linear correlation with NpNn for each case, as was shown in Fig. 1 (c) of Ref. [10]. We note without details that one obtains a similar pattern if one replaces results of Ref. [19] in Fig. 1 (a-d) by using those of Refs. [20] and [21], i.e., the Duflo-Zuker model and the finite-range-liquid-drop model. Below, this pattern is attributed to symmetry energy with the shell correction.

    Figure 1

    Figure 1.  (color online) VNP versus NpNn for the (28<Z<50, 28<N<50), (28<Z<50, 50<N<82), (50<Z<82, 50<N<82),and (50<Z<82, 82<N<126) major shells. Panels (a-d) are extracted from binding energies of Ref. [19] [i.e., the WS3 model] by using Eq. (1), and panels (a-d) are calculated by using Eq. (16). One sees that the results of these two approaches are consistent with each other. We note without details that one obtains similar results if one replaces results of Ref. [19] by using those of Refs. [20] and [21], i.e., the Duflo-Zuker model and the finite-range-liquid-drop model.

    We take the Bethe-Weizsäcker formula in the form of Ref. [19]:

    B(N,Z)=avAasA23acZ2A13(10.76Z23)cVsymI2A+cSsymI2A2/3apairA13δnp+BW+Bshell,

    (3)

    where av,as,ac,cVsym,cSsym, and apair are coefficients corresponding to the volume energy, surface energy, coulomb energy, volume symmetry energy, surface symmetry energy, and pairing energy, and δnp is the same as in Ref. [19]. For these terms, we adopt the same parameters presented in Table I of Ref. [19] (it is noted that variations of these parameters do not change the pattern of this paper, as will be seen below). The last two terms, i.e., BW and Bshell, correspond to the Wigner term and the shell correction term, respectively. One sees easily that the volume energy term is canceled out in Eq. (1) and does not contribute to VNP. Therefore, in this paper, we skip this term, although it is actually the most important part of the binding energy in the liquid drop model.

    We denote the contributions of the surface energy, Coulomb energy, pairing terms, symmetry energy, Wigner energy, and shell correction to VNP as VsurfaceNP, VCoulombNP, VpairNP, VsymNP, VWNP, and VshNP, respectively. To proceed with our discussion, we assume NpZ0+N01 and NnZ0+N01. These assumptions are reasonably good unless the mass number A=Z+N is small; for the four major shells that we discuss in this paper, and particularly for heavy nuclei, these assumptions are applicable.

    Now, we show that the sum of these VsymNP, VsurfaceNP, VCoulombNP, and VpairNP terms yields a linear correlation with NpNn as the leading order. We note, without details, that these formulas are in unified form for particle-particle, hole-hole, particle-hole, and hole-particle cases, because we take the valence nucleon number to be the number of holes for major shells that are more than half-filled, as indicated by Eqs. (1)–(2).

    Because the derivations of VsymNP, VsurfaceNP, VCoulombNP, and VpairNP are cumbersome, we present the details in Appendix A, except for VsymNP, i.e., the dominant part in VNP. In Eq. (3), the symmetry energy is given by two terms:

    cVsymI2A+cSsymI2A2/3.

    (4)

    Correspondingly, VsymNP has two terms, which are denoted as [VsymNP]V and [VsymNP]S. By using Eqs. (1)–(2), we obtain

    [VsymNP]V=14[cVsym(NZ)2N+ZcVsym(NZ)2N+Z+2cVsym(NZ+1)2N+Z+1cVsym(NZ1)2N+Z+1cVsym(N0Z0)2N0+Z0cVsym(N0Z0)2N0+Z0+2cVsym(N0Z0+1)2N0+Z0+1cVsym(N0Z01)2N0+Z0+1+cVsym(NZ0)2N+Z0+cVsym(NZ0)2N+Z0+2+cVsym(NZ0+1)2N+Z0+1+cVsym(NZ01)2N+Z0+1+cVsym(N0Z)2N0+Z+cVsym(N0Z)2N0+Z+2+cVsym(N0Z+1)2N0+Z+1+cVsym(N0Z1)2N0+Z+1].

    (5)

    As an approximation, we assume that N+Z, N0+Z0, N0+Z, and N+Z0 plus 0 (1 or 2) in the denominators on the right-hand side of the above formula are equal to (N+N0+Z+Z0)/2. The above [VsymNP]V is reduced to

    [VsymNP]V12cVsymN+N0+Z+Z0[(NZ)2(NZ)2(NZ+1)2(NZ1)2(N0Z0)2(N0Z0)2(N0Z0+1)2(N0Z01)2+(NZ0)2+(NZ0)2+(NZ0+1)2+(NZ01)2+(N0Z)2+(N0Z)2+(N0Z+1)2+(N0Z1)2].

    (6)

    By substituting N=N0+Nn and Z=Z0+Np on the right-hand side of the above formula, we easily obtain

    [VsymNP]V4cVsymN+N0+Z+Z0NpNn.

    Similarly, one obtains

    [VsymNP]S27/3cSsymN+N0+Z+Z0NpNn.

    Therefore, we obtain

    VsymNP2NpNn[2cVsymN+N0+Z+Z024/3cSsym(N+N0+Z+Z0)4/3].

    (7)

    Similarly, we obtain

    VsurfaceNP29as1(Z0+N0)4/3NpNn,

    (8)

    VCoulombNPac[23Z0(Z0+N0)4/349Z20(Z0+N0)7/3]NpNn+0.76ac[49Z1/30(Z0+N0)4/3+49Z4/30(Z0+N0)7/3]NpNn,

    (9)

    VpairNPapair[491(Z0+N0)7/3+79N0Z0(Z0+N0)103]NpNn.

    (10)

    Here, the first term on the right-hand side of Eq. (9) comes from the direct term and the second term comes from the exchange term in the Coulomb energy. According to Fig. 2, the values of VCoulombNP are maximally 10 MeV and are far smaller than the values of VsymNP, and more importantly, their values for the particle-particle, hole-hole, particle-hole, and hole-particle cases, are very close to each other. Therefore, the inclusion of this term would not yield any essential differences in the regular pattern of VNP. The values of VsurfaceNP and VpairNP are always very small, and we do not consider them below in this paper.

    Figure 2

    Figure 2.  (color online) VSymNP, VSurfaceNP, and VCoulombNP calculated by using Eqs. (7)–(9), respectively, versus NpNn. We note without details that the magnitude of VpairingNP is close to zero, and it is omitted here. One sees clearly that the magnitude of VSymNP is far larger than those of VSurfaceNP and VCoulombNP.

    The results of Eqs. (7)–(10) are very interesting, because all these contributions to the integrated neutron-proton interaction, which originated from the symmetry, surface, Coulomb and pairing energies in the mass formula of the liquid-drop model, are dominantly linear versus NpNn. This provides us with a simple explanation of the good correlation between VNP and NpNn, which was explored in the literature [810].

    In Fig. 2, we plot VsymNP, VsurfaceNP, and VCoulombNP for the case of the major shells of 82<N<126 and 50<Z<82. VpairNP is not plotted, because its value is always close to zero. From this figure, one sees that the contribution of VsymNP is dominant, while the two other contributions, i.e., those of VCoulombNP and VsurfaceNP, are far smaller. In fact, the relevance measurement of these terms can be clearly seen from Eqs. (7)–(10), where the ratios to NpNn for VsymNP, VsurfaceNP, VCoulombNP, and VpairNP, are approximately proportional to 1/A, 1/A4/3, 1/A4/3, and 1/A7/3, respectively.

    In this section we discuss contributions from other two "residual" terms of binding energy in the liquid drop model: the Wigner energy term and the shell correction term in Eq. (3).

    The contribution to VNP from the Wigner energy is sizable only for the particle-particle or hole-hole case with valence protons and neutrons in the same major shells; otherwise, this contribution is very small and is negligible (mostly below 1 MeV) in comparison with the value of VNP, similar to the situation of VpairNP, and this is the case for the (50<Z<82, 82<N<126) shell. In this paper, for the sake of completeness, we investigate the particle-particle or hole-hole case with valence protons and neutrons in the same major shells.

    We assume that (Np+Nn)/(N+Z) is small and expand the contribution from the Wigner energy in terms of this ratio. For simplicity, we adopt the Wigner energy from Ref. [22]:

    Bw(Z,N)=W|NZ|Ad1AδN,Zπnp,

    (11)

    where W=42.7 MeV and d=28.7 MeV, according to Ref. [22]. We note that the results are very close to those obtained by assuming the Wigner energy of Refs. [19], without details. Here, πnp equals 1 for odd-odd nuclei and vanishes otherwise.

    Correspondingly, the contribution to VNP from the Wigner energy has two terms, which are denoted as VWNP and VdNP, respectively. The result of VdNP is simple and takes the following form. When N and Z are even and N=Z,

    VdNP=d4[1A0+21A+2];

    (12)

    and when N and Z are odd and N=Z,

    VdNP=d4[1A0+21A];

    (13)

    VdNP vanishes otherwise. From these results, one easily sees that VdNP is negligibly small in comparison with the value of VNP in all the regions that we discuss in this paper. For simplicity, one assumes VdNP0. The details of deriving VWNP are presented in Appendix A of this paper, and the final results are as follows. When the proton and neutron are in the same major shells,

    VWNP4WN+Z+2N0min(Np,Nn)

    (14)

    for the particle-particle case and

    VWNP4WN+Z+2N0min(Np,Nn)

    (15)

    for the hole-hole case [in Eq. (15), Np and Nn correspond to the numbers of holes]. According to the above two formulas, VWNP is proportional to Np (or Nn) when Np (or Nn) is smaller than Nn (or Np). Although the VWNP values in Eqs. (14)–(15) are not well linear-correlated with NpNn, they increase as Np and/or Nn increase. Furthermore, the values of VWNP are maximally approximately 10 MeV for the particle-particle and hole-hole cases when the proton and neutron are in the same major shell and thus are far smaller than VsymNP. In principle, VWNP breaks the linearity between VNP and NpNn in these two special cases, but this breaking is minor. We note again that the contribution of the Wigner energy to VNP is negligible when one investigates the (28<Z<50, 50<N<82) and (50<Z<82, 82<N<126) major shells, in which cases valence protons and neutrons are not in the same major shells.

    We finally come to the VshNP term, by adopting the calculated Bshell of Ref. [19]. The results for VshNP are plotted in terms of NpNn in Fig. 3. One sees that these VshNP values exhibit reasonable linearity with NpNn in most cases (with fluctuations), with the exception of the (50<Z<82, 82<N<126) major shells in which the magnitudes of VshNP increase when NpNn is below 100 and tend to be saturated when NpNn is larger than 100. However, all these VshNP values are far smaller than the corresponding VsymNP results. Additionally, the VshNP values of the hole-hole case are maximally approximately 12 MeV (positive), and those of the particle-hole case are maximally approximately 7 MeV (negative). We shall see soon that the sizable differences of VshNP between the hole-hole case and particle-hole (hole-particle) case are very important for explaining the subtle pattern of VNP versus NpNn, as observed in Refs. [10, 11].

    Figure 3

    Figure 3.  (color online) The contribution to VNP from the shell correction part in the liquid drop model, for four major shells. Here, the shell correction energies are taken from the WS3 model.

    In this section, we discuss the implication of our derived formula for VNP.

    By summing all the above results of Eqs. (7)–(15), neglecting contributions from the Coulomb energy and pairing interaction [when one discusses the (28<Z<50, 50<N<82) and (50<Z<82, 82<N<126) major shells, the term VWNP is also negligible], the neutron-proton interactions are essentially given by

    VNPVsymNP+VshNP+VWNP.

    (16)

    By using Eq. (16), VsymNP of Eq. (7), the VshNP extracted by the shell correction results of Ref. [19], and VWNP of Eqs. (14) and (15), we obtain VNP and plot it versus NpNn in panels (a-d) of Fig. 1(labeled as "this work"). One sees good agreement with the results in panels (a-d).

    It is interesting and also one of the purposes of this paper to explain subtle details of the pattern exhibited in Fig. 1. This pattern is very striking and well-known for nuclei in the (28<Z<50,50<N<82) and (50<Z<82, 82<N<126) major shells, for which Eq. (16) is reduced to

    VNPVsymNP+VshNP,

    (17)

    assuming that both VCoulombNP0 and VWNP0. Because the ratio of VsymNP to NpNn is dominantly of 1/A-dependence according to Eq. (7), the neutron-proton interaction is strongest for the particle-particle case, for which the mass number is the smallest among the four cases, i.e., particle-particle, particle-hole, hole-particle, and hole-hole. One therefore expects the ordering of VNP as follows. The VNP of the particle-particle case is the largest, that of the hole-hole case is the smallest, and that of the particle-hole and hole-particle cases is in-between.

    Interestingly, the above simple pattern is actually "refined", albeit slightly, by the VshNP term. This refinement is striking in particular for the (28<Z<50, 50<N<82) and (50<Z<82, 82<N<126) major shells. As shown in Fig. 3 and discussed in Sec. III, the VshNP values are positive for both the particle-particle and hole-hole cases and are negative for both the hole-particle and particle-hole cases. Therefore, the neutron-proton interactions for the particle-particle case is further enhanced by VshNP and thus is the largest among the four cases, i.e., the particle-particle, hole-hole, particle-hole, and hole-particle cases. For the particle-hole case and the hole-hole case of the (50<Z<82, 82<N<126) major shells, although the VsymNP results of the hole-hole case are the smallest, they are "lifted" up by approximately 12 MeV maximally, while the VsymNP results of the particle-hole case are reduced by maximally approximately 7 MeV. This competition is the key to explain the order inversion of VNP for the particle-hole and hole-hole cases. It is the term VshNP that reduces VNP for the particle-hole case and boosts VNP for the hole-hole case, thus yielding the order inversion of VNP for these two cases. This is precisely the pattern reported in Refs. [10, 11].

    To summarize, in this paper, we study the patterns of neutron-proton interactions (denoted by VNP) in a few major shells of the nuclide chart: (28<Z<50, 28<N<50), (28<Z<50, 50<N<82), (50<Z<82, 50<N<82), and (50<Z<82, 82<N<126). We show that the dominant part in VNP originates from the symmetry energy, whose contribution is approximately proportional to NpNn, i.e., the product of the valence proton number and valence neutron number. We note without details that this pattern is robust; i.e., one obtains essentially the same pattern if one replaces results of Ref. [19] by using those of Refs. [20] and [21], i.e., the Duflo-Zuker model and the finite-range-liquid-drop model.

    Contributions to the VNP from other parts in the liquid-drop model, such as the volume energy, surface energy term, and Coulomb energy term, are either zero or close to zero. The contribution from the Wigner energy is either very close to zero (when valence protons and neutrons are not in the same major shells) or far smaller than that from the symmetry energy term. The VNP values of these origins are demonstrated to be the largest for the particle-particle case and the smallest for the hole-hole case. However, the contribution to the VNP from the shell correction is positive for particle-particle and hole-hole cases and is negative for particle-hole and hole-particle cases. Therefore one has always the strongest VNP of the particle-particle case for all major shells. The competition of VsymNP, which is the smallest for the hole-hole case and in-between for the particle-hole and hole-particle cases, with VshNP, which is positive for the hole-hole case and negative for the particle-hole and hole-particle cases, yields an order inversion of VNP for the hole-hole and particle-hole cases, as observed in previous papers [10, 11].

    In the Appendix, we present the details to derive Eqs. (8)–(10), (14), and (15). We exemplify the derivations of the four cases, i.e., the particle-particle, hole-hole, particle-hole, and hole-particle cases, by using the particle-particle case only, as it would be redundant and tedious to present all four cases. The formulas for the other three cases can be obtained in the same way, and with the same form. The particle-particle case corresponds to δp=δn=1 in Eq. (1). The contributions of the different components to VNP, including VsymNP, VsurfaceNP, VCoulombNP, VpairNP, and VWNP, include 16 terms, according to the definition of the empirical VNP in Eqs. (1)–(2). In Sec. II, we present the derivation of [VsymNP]V.

    We first come to the VsurfaceNP term, with the surface energy of the mass formula defined by asA23. From the definition of VNP in Eqs. (1)–(2), we have

    VsurfaceNP=14[as(Z+N)2/3as(Z+N+2)2/3as(Z+N+1)2/3as(Z+N+1)2/3as(Z0+N0)2/3as(Z0+N0+2)2/3as(Z0+N0+1)2/3as(Z0+N0+1)2/3+as(Z0+N)2/3+as(Z0+N+2)2/3+as(Z0+N+1)2/3+as(Z0+N+1)2/3+as(Z+N0)2/3+as(Z+N0+2)2/3+as(Z+N0+1)2/3+as(Z+N0+1)2/3].

    By using the convention A0=N0+N0, Z=Z0+Np, and N=N0+Nn, the above formula is rewritten as follows:

    VsurfaceNP=14asA2/30[(1+Np+NnA0)2/3(1+Np+Nn+2A0)2/32(1+Np+Nn+1A0)2/31(1+2A0)2/32(1+1A0)2/3+(1+NnA0)2/3+(1+Nn+2A0)2/3+2(1+Nn+1A0)2/3+(1+NpA0)2/3+(1+Np+2A0)2/3+2(1+Np+1A0)2/3].

    We expand the right-hand side of VsurfaceNP in terms of Np/A0 and Nn/A0 and obtain

    VsurfaceNP14as[29+49[1+1/(Z0+N0)]4/3+29[1+2/(Z0+N0)]4/3]NpNn(Z0+N0)4/329asNpNn(Z0+N0)4/3.

    This gives Eq. (8).

    We next come to the contribution of Coulomb energy to VNP. We use the Coulomb energy in the mass formula to be acZ2A13(10.76Z23). Here, the contribution from the first term is called the direct term, which is denoted as[VCoulombNP]d. As in VsurfaceNP, [VCoulombNP]d has also 16 terms and can be written as follows.

    [VCoulombNP]d=14acA5/30×[(Z0+NpA0)2(1+Np+NnA0)1/3(Z0+Np+1A0)2(1+Np+Nn+2A0)1/3(Z0+Np+1A0)2(1+Np+Nn+1A0)1/3(Z0+NpA0)2(1+Np+Nn+1A0)1/3(Z0A0)2(Z0+1A0)2(1+2A0)1/3(Z0+1A0)2(1+1A0)1/3(Z0A0)2(1+1A0)1/3+(Z0A0)2(1+NnA0)1/3+(Z0+1A0)2(1+Nn+2A00)1/3+(Z0+1A0)2(1+Nn+1A0)1/3+(Z0A0)2(1+Nn+1A0)1/3+(Z0+NpA0)2(1+NpA0)1/3+(Z0+Np+1A0)2(1+Np+2A0)1/3+(Z0+Np+1A0)2(1+Np+1A0)1/3+(Z0+NpA0)2(1+Np+1A0)1/3].

    We expand all these terms in terms of NpA0 and NnA0, yielding

    [VCoulombNP]d14ac(A0)5/3[2Z0A03(1+1A0)4/34(Z0A0)29(1+1A0)7/3+2(3+12Z0A0)(1+Z0A0)9(1+1A0)7/3+2(4+42Z0A0)(1+Z0A0)9(1+2A0)7/329(3Z0A0+2(Z0A0)2)]1(A0)2NpNnac[23Z0(Z0+N0)4/349Z20(Z0+N0)7/3]NpNn.

    This gives the first term of Eq. (9). The second term in Eq. (9) is obtained in the same way.

    In Eqs. (1)–(3), the definition of the pairing energy is

    Bpair(Z,N)=apairA13δnp.

    Here, δnp is defined as

    δnp={2|I|: {\it N} and {\it Z} even|I|: {\it N} and {\it Z} odd1|I|: {\it N} even, {\it Z} odd, and {\it N} > {\it Z} 1|I|: {\it N} odd, {\it Z} even, and {\it N} < {\it Z} 1: {\it N} even, {\it Z} odd, and {\it N} < {\it Z} 1: {\it N} odd, {\it Z} even, and {\it N} > {\it Z} ,

    with isospin asymmetry I=(NZ)/A. As an approximation, we assume that (N+Z+1)1/3 and (N+Z+1)1/3 are equal to (N+Z)1/3; NZN+Z+2 and NZ+1N+Z+1 are equal to (NZ)N+Z, and to exemplify the derivation of VpairNP with N>Z and both (Z, N) odd, we have

    VpairNPapair[(N+Z)1/3(4|NZ|N+Z)+(N0+Z0)1/3(4|N0Z0|N0+Z0)(N0+Z)1/3(4|N0Z|N0+Z)(N+Z0)1/3(4|NZ0|N+Z0)]apair[491(Z0+N0)7/3+79N0Z0(Z0+N0)103]NpNn,

    This gives Eq. (10) for the N>Z case. In all cases of Eq. (23), VpairNP is negligibly small in the VNP-NpNn plot.

    The Wigner energy is defined in Eq. (11). The contribution to the VNP from the second term is very simple and is given by Eqs. (12)–(13). The contribution from the first term, i.e., W|NZ|A, has 16 terms, which can be simplified by using the assumption that N+Z, N0+Z0, N0+Z, and N+Z0 plus 0 or 1 or 2 in the denominators equal (N+N0+Z+Z0)/2. We have

    VWNPW2(N+N0+Z+Z0)[2|NZ||NZ+1||NZ1|2|N0Z0||N0Z0+1||N0Z01|+2|NZ0|+|NZ0+1|+|NZ01|+2|N0Z|+|N0Z+1|+|N0Z1|].

    In most cases, NZ1, and under this assumption, one has

    VWNP2WN+N0+Z+Z0[|NZ||N0Z0|+|NZ0|+|N0Z|].

    Clearly, as expected, when valence protons and neutrons are not in the same major shells or when valence protons and neutrons are in the same major shells for the particle-hole and hole-particle cases, VWNP and VWNP equal zero in the above formula (in the realistic case, they are very close to zero). For the particle-particle case with valence protons and neutrons in the same major shells, one has

    VWNP4WN+Z+2N0(min{N,Z}N0);

    for the hole-hole case with valence protons and neutrons in the same major shells,

    VWNP4WN+Z+2N0(N0max{N,Z}).

    The above two formulas give Eqs. (14)–(15).

    [1] A. De Shalit and M. Goldhaber, Phys. Rev. 92, 1211 (1953) doi: 10.1103/PhysRev.92.1211
    [2] I. Talmi, Rev. Mod. Phys. 34, 704 (1962) doi: 10.1103/RevModPhys.34.704
    [3] P. Federman and S. Pittel, Phys. Lett. B 69, 385 (1977) doi: 10.1016/0370-2693(77)90825-5
    [4] P. Federman, S. Pittel, and R. Campas, Phys. Lett. B 82, 9 (1979) doi: 10.1016/0370-2693(79)90412-X
    [5] R. F. Casten, Phys. Rev. Lett. 54, 1991 (1985) doi: 10.1103/PhysRevLett.54.1991
    [6] R. F. Casten and N.V. Zamfir, J. Phys. G 22, 1521 (1996) doi: 10.1088/0954-3899/22/11/002
    [7] R. F. Casten, Nuclear Structure From a Simple Perspective (Oxford Science Pulications, 2000)
    [8] J. Y. Zhang, R. F. Casten, and D. S. Brenner, Phys. Lett. B 227, 1 (1989) doi: 10.1016/0370-2693(89)91273-2
    [9] G. J. Fu, H. Jiang, Y. M. Zhao et al., Phys. Rev. C 82, 014307 (2010) doi: 10.1103/PhysRevC.82.014307
    [10] M. Q. Lin, C. Ma, and Y. M. Zhao, Phys. Rev. C 105, L021305 (2022) doi: 10.1103/PhysRevC.105.L021305
    [11] R. B. Cakirli and R. F. Casten, Phys. Rev. Lett. 96, 132501 (2006) doi: 10.1103/PhysRevLett.96.132501
    [12] M. Stoitsov, R. B. Cakirli, R. F. Casten et al., Phys. Rev. Lett. 98, 132502 (2007) doi: 10.1103/PhysRevLett.98.132502
    [13] W. Satula, R. A. Wyss, and M. Rafalski, Phys. Rev. C 74, 011301(R) (2006) doi: 10.1103/PhysRevC.74.011301
    [14] P. -G. Reinhard, M. Bender, W. Nazarewicz et al., Phys. Rev. C 73, 014309 (2006) doi: 10.1103/PhysRevC.73.014309
    [15] W. Satula, D. J. Dean, J. Gary et al., Phys. Lett. B 407, 103 (1997) doi: 10.1016/S0370-2693(97)00711-9
    [16] D. Bonatsos, S. Karampagia, R. B. Cakirli et al., Phys. Rev. C 88, 054309 (2013) doi: 10.1103/PhysRevC.88.054309
    [17] R. F. Casten and R. B. Cakirli, Phys. Scr. 91, 033004 (2016) doi: 10.1088/0031-8949/91/3/033004
    [18] Z. Wu, S. A. Changizi, and Chong Qi, Phys. Rev. C 93, 034334 (2016) doi: 10.1103/PhysRevC.93.034334
    [19] M. Liu, N. Wang, Y. G. Deng et al., Phys. Rev. C 84, 014333 (2011) doi: 10.1103/PhysRevC.84.014333
    [20] J. Duflo and A. P. Zuker, Phys. Rev. C 52, R23(R) (1995) doi: 10.1103/PhysRevC.52.R23
    [21] P. Möller, W. D. Myers, H. Sagawa et al., Phys. Rev. Lett. 108, 052501 (2012) doi: 10.1103/PhysRevLett.108.052501
    [22] Y. Y. Cheng, M. Bao, Y. M. Zhao et al., Phys. Rev. C 91, 024313 (2015) doi: 10.1103/PhysRevC.91.024313
  • [1] A. De Shalit and M. Goldhaber, Phys. Rev. 92, 1211 (1953) doi: 10.1103/PhysRev.92.1211
    [2] I. Talmi, Rev. Mod. Phys. 34, 704 (1962) doi: 10.1103/RevModPhys.34.704
    [3] P. Federman and S. Pittel, Phys. Lett. B 69, 385 (1977) doi: 10.1016/0370-2693(77)90825-5
    [4] P. Federman, S. Pittel, and R. Campas, Phys. Lett. B 82, 9 (1979) doi: 10.1016/0370-2693(79)90412-X
    [5] R. F. Casten, Phys. Rev. Lett. 54, 1991 (1985) doi: 10.1103/PhysRevLett.54.1991
    [6] R. F. Casten and N.V. Zamfir, J. Phys. G 22, 1521 (1996) doi: 10.1088/0954-3899/22/11/002
    [7] R. F. Casten, Nuclear Structure From a Simple Perspective (Oxford Science Pulications, 2000)
    [8] J. Y. Zhang, R. F. Casten, and D. S. Brenner, Phys. Lett. B 227, 1 (1989) doi: 10.1016/0370-2693(89)91273-2
    [9] G. J. Fu, H. Jiang, Y. M. Zhao et al., Phys. Rev. C 82, 014307 (2010) doi: 10.1103/PhysRevC.82.014307
    [10] M. Q. Lin, C. Ma, and Y. M. Zhao, Phys. Rev. C 105, L021305 (2022) doi: 10.1103/PhysRevC.105.L021305
    [11] R. B. Cakirli and R. F. Casten, Phys. Rev. Lett. 96, 132501 (2006) doi: 10.1103/PhysRevLett.96.132501
    [12] M. Stoitsov, R. B. Cakirli, R. F. Casten et al., Phys. Rev. Lett. 98, 132502 (2007) doi: 10.1103/PhysRevLett.98.132502
    [13] W. Satula, R. A. Wyss, and M. Rafalski, Phys. Rev. C 74, 011301(R) (2006) doi: 10.1103/PhysRevC.74.011301
    [14] P. -G. Reinhard, M. Bender, W. Nazarewicz et al., Phys. Rev. C 73, 014309 (2006) doi: 10.1103/PhysRevC.73.014309
    [15] W. Satula, D. J. Dean, J. Gary et al., Phys. Lett. B 407, 103 (1997) doi: 10.1016/S0370-2693(97)00711-9
    [16] D. Bonatsos, S. Karampagia, R. B. Cakirli et al., Phys. Rev. C 88, 054309 (2013) doi: 10.1103/PhysRevC.88.054309
    [17] R. F. Casten and R. B. Cakirli, Phys. Scr. 91, 033004 (2016) doi: 10.1088/0031-8949/91/3/033004
    [18] Z. Wu, S. A. Changizi, and Chong Qi, Phys. Rev. C 93, 034334 (2016) doi: 10.1103/PhysRevC.93.034334
    [19] M. Liu, N. Wang, Y. G. Deng et al., Phys. Rev. C 84, 014333 (2011) doi: 10.1103/PhysRevC.84.014333
    [20] J. Duflo and A. P. Zuker, Phys. Rev. C 52, R23(R) (1995) doi: 10.1103/PhysRevC.52.R23
    [21] P. Möller, W. D. Myers, H. Sagawa et al., Phys. Rev. Lett. 108, 052501 (2012) doi: 10.1103/PhysRevLett.108.052501
    [22] Y. Y. Cheng, M. Bao, Y. M. Zhao et al., Phys. Rev. C 91, 024313 (2015) doi: 10.1103/PhysRevC.91.024313
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X. Yin and M. Zhao. Simple scenario of integrated neutron-proton interaction[J]. Chinese Physics C. doi: 10.1088/1674-1137/acc5dd
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Simple scenario of integrated neutron-proton interaction

  • 1. Shanghai Key Laboratory of Particle Physics and Cosmology, School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China
  • 2. Collaborative Innovation Center of IFSA (CICIFSA), Shanghai Jiao Tong University, Shanghai 200240, China

Abstract: In this study, we investigate the patterns exhibited by integrated neutron-proton interactions (denoted as VNP) that exhibit systematic differences among particle-particle, hole-hole, hole-particle, and particle-hole cases. A simple formula of VNP is proposed to be in approximate linearity with NnNp. This formula yields regular patterns of VNP that are highly consistent with those previously extracted according to binding energies. The observed ordering of VNP, i.e., VNP of the particle-particle case is the largest, VNP of the hole-hole case is in-between, and VNP of the particle-hole and hole-particle cases is the smallest, is explained in terms of the dominant part of VNP originating from symmetry energy and refinement involving the shell correction in the mass formulas.

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    I.   INTRODUCTION
    • Neutron-proton interactions play the most important role in the evolution of the shell structure, collectivity, phase shape transitions, and deformation, as stressed by de Shalit [1] and Talmi [2] and later by Federman and Pittel [3, 4]. The neutron-proton interaction was simplified and parametrized as NpNn, i.e., the product of the valence proton number and valence neutron number, by Casten [5]. This is called the NpNn scheme in literature, or in a more semantic meaning, the valence correlation scheme [6, 7]. Zhang and collaborators [8], and later Fu et al. [9], empirically extracted integrated neutron-proton interactions (denoted as VNP) by using the experimental atomic masses, and a remarkable linearity between VNP and NpNn was shown for the case with 50<Z<82 and 50<N<82. Recently, it was demonstrated [10] that such integrated neutron-proton interactions exhibit systematic differences for the particle-particle, hole-hole, and particle-hole cases in the (50<Z<82 and 82<Z<126) major shells. This pattern is a reflection of the differences in the average neutron-proton interactions of those three cases, as pointed out earlier by Cakirli and Casten in Ref. [11]. For completeness, we mention Refs. [1218], in which neutron-proton interactions were also studied from other perspectives.

      The purpose of this paper is to provide a simple scenario for the above interesting pattern of integrated neutron-proton interactions. We show that these regularities essentially originate from nuclear symmetry energy, with a subtle effect from the shell correction. We also present a compact formula of VNP in terms of NnNp.

      The remainder of this paper is organized as follows. In Sec. II, we derive the formula of VNP based on the improved liquid-drop model with the shell correction [19]. In Sec. III, we discuss the contributions of the Wigner energy and the shell effect to the VNP, and in Sec. IV, we discuss the linear correlation between VNP and NpNn as well as the relative magnitudes of the particle-particle, hole-hole, particle-hole, and hole-particle cases. In Sec. V, we summarize this paper.

    II.   NEUTRON-PROTON INTERACTIONS AND SYMMETRY ENERGY
    • In this section, we present the values of VNP extracted by using theoretical binding energies of the WS3 model [19] and compare these empirical results for VNP with those calculated via our simple formula of VNP derived from the liquid-drop model with the shell correction. We shall see remarkable consistency between VNP values obtained via these two approaches.

      Let us begin our discussion with the definition of VNP. According to Eqs. (4)–(5) of Ref. [9], the empirical integrated neutron-proton interaction is expressed as follows:

      VNP(Z,N)=14δpδn[S(Z,N)+S(Z0,N0)S(Z0,N)S(Z,N0)],

      (1)

      where δp (δn) is +1 if the valence protons (neutrons) are particle-like and 1 if the valence protons (neutrons) are hole-like, Z0 (N0) is the nearest magic number for protons (neutrons), and S(Z,N) is defined as

      S(Z,N)=B(Z+δp,N+δn)+B(Z+δp,N)+B(Z,N+δn)+B(Z,N),

      (2)

      where B represents the nuclear binding energy. For convenience, in this paper, we use the convention that the values of B are positive; with this convention, the values of VNP are positive.

      In Fig. 1, we plot such extracted VNP values versus NpNn from the improved Weizsäcker mass formula (WS3) [19] for numerous major shells: (28<Z<50, 28<N<50), (28<Z<50, 50<N<82), (50<Z<82, 50<N<82), and (50<Z<82, 82<N<126). These empirical neutron-proton interactions are plotted in panels (a-d), with blue color for the particle-particle case, red for the hole-hole case, green for the particle-hole case, and violet for the hole-particle case. One also sees that the extracted VNP values have a good linear correlation with NpNn for each case, as was shown in Fig. 1 (c) of Ref. [10]. We note without details that one obtains a similar pattern if one replaces results of Ref. [19] in Fig. 1 (a-d) by using those of Refs. [20] and [21], i.e., the Duflo-Zuker model and the finite-range-liquid-drop model. Below, this pattern is attributed to symmetry energy with the shell correction.

      Figure 1.  (color online) VNP versus NpNn for the (28<Z<50, 28<N<50), (28<Z<50, 50<N<82), (50<Z<82, 50<N<82),and (50<Z<82, 82<N<126) major shells. Panels (a-d) are extracted from binding energies of Ref. [19] [i.e., the WS3 model] by using Eq. (1), and panels (a-d) are calculated by using Eq. (16). One sees that the results of these two approaches are consistent with each other. We note without details that one obtains similar results if one replaces results of Ref. [19] by using those of Refs. [20] and [21], i.e., the Duflo-Zuker model and the finite-range-liquid-drop model.

      We take the Bethe-Weizsäcker formula in the form of Ref. [19]:

      B(N,Z)=avAasA23acZ2A13(10.76Z23)cVsymI2A+cSsymI2A2/3apairA13δnp+BW+Bshell,

      (3)

      where av,as,ac,cVsym,cSsym, and apair are coefficients corresponding to the volume energy, surface energy, coulomb energy, volume symmetry energy, surface symmetry energy, and pairing energy, and δnp is the same as in Ref. [19]. For these terms, we adopt the same parameters presented in Table I of Ref. [19] (it is noted that variations of these parameters do not change the pattern of this paper, as will be seen below). The last two terms, i.e., BW and Bshell, correspond to the Wigner term and the shell correction term, respectively. One sees easily that the volume energy term is canceled out in Eq. (1) and does not contribute to VNP. Therefore, in this paper, we skip this term, although it is actually the most important part of the binding energy in the liquid drop model.

      We denote the contributions of the surface energy, Coulomb energy, pairing terms, symmetry energy, Wigner energy, and shell correction to VNP as VsurfaceNP, VCoulombNP, VpairNP, VsymNP, VWNP, and VshNP, respectively. To proceed with our discussion, we assume NpZ0+N01 and NnZ0+N01. These assumptions are reasonably good unless the mass number A=Z+N is small; for the four major shells that we discuss in this paper, and particularly for heavy nuclei, these assumptions are applicable.

      Now, we show that the sum of these VsymNP, VsurfaceNP, VCoulombNP, and VpairNP terms yields a linear correlation with NpNn as the leading order. We note, without details, that these formulas are in unified form for particle-particle, hole-hole, particle-hole, and hole-particle cases, because we take the valence nucleon number to be the number of holes for major shells that are more than half-filled, as indicated by Eqs. (1)–(2).

      Because the derivations of VsymNP, VsurfaceNP, VCoulombNP, and VpairNP are cumbersome, we present the details in Appendix A, except for VsymNP, i.e., the dominant part in VNP. In Eq. (3), the symmetry energy is given by two terms:

      cVsymI2A+cSsymI2A2/3.

      (4)

      Correspondingly, VsymNP has two terms, which are denoted as [VsymNP]V and [VsymNP]S. By using Eqs. (1)–(2), we obtain

      [VsymNP]V=14[cVsym(NZ)2N+ZcVsym(NZ)2N+Z+2cVsym(NZ+1)2N+Z+1cVsym(NZ1)2N+Z+1cVsym(N0Z0)2N0+Z0cVsym(N0Z0)2N0+Z0+2cVsym(N0Z0+1)2N0+Z0+1cVsym(N0Z01)2N0+Z0+1+cVsym(NZ0)2N+Z0+cVsym(NZ0)2N+Z0+2+cVsym(NZ0+1)2N+Z0+1+cVsym(NZ01)2N+Z0+1+cVsym(N0Z)2N0+Z+cVsym(N0Z)2N0+Z+2+cVsym(N0Z+1)2N0+Z+1+cVsym(N0Z1)2N0+Z+1].

      (5)

      As an approximation, we assume that N+Z, N0+Z0, N0+Z, and N+Z0 plus 0 (1 or 2) in the denominators on the right-hand side of the above formula are equal to (N+N0+Z+Z0)/2. The above [VsymNP]V is reduced to

      [VsymNP]V12cVsymN+N0+Z+Z0[(NZ)2(NZ)2(NZ+1)2(NZ1)2(N0Z0)2(N0Z0)2(N0Z0+1)2(N0Z01)2+(NZ0)2+(NZ0)2+(NZ0+1)2+(NZ01)2+(N0Z)2+(N0Z)2+(N0Z+1)2+(N0Z1)2].

      (6)

      By substituting N=N0+Nn and Z=Z0+Np on the right-hand side of the above formula, we easily obtain

      [VsymNP]V4cVsymN+N0+Z+Z0NpNn.

      Similarly, one obtains

      [VsymNP]S27/3cSsymN+N0+Z+Z0NpNn.

      Therefore, we obtain

      VsymNP2NpNn[2cVsymN+N0+Z+Z024/3cSsym(N+N0+Z+Z0)4/3].

      (7)

      Similarly, we obtain

      VsurfaceNP29as1(Z0+N0)4/3NpNn,

      (8)

      VCoulombNPac[23Z0(Z0+N0)4/349Z20(Z0+N0)7/3]NpNn+0.76ac[49Z1/30(Z0+N0)4/3+49Z4/30(Z0+N0)7/3]NpNn,

      (9)

      VpairNPapair[491(Z0+N0)7/3+79N0Z0(Z0+N0)103]NpNn.

      (10)

      Here, the first term on the right-hand side of Eq. (9) comes from the direct term and the second term comes from the exchange term in the Coulomb energy. According to Fig. 2, the values of VCoulombNP are maximally 10 MeV and are far smaller than the values of VsymNP, and more importantly, their values for the particle-particle, hole-hole, particle-hole, and hole-particle cases, are very close to each other. Therefore, the inclusion of this term would not yield any essential differences in the regular pattern of VNP. The values of VsurfaceNP and VpairNP are always very small, and we do not consider them below in this paper.

      Figure 2.  (color online) VSymNP, VSurfaceNP, and VCoulombNP calculated by using Eqs. (7)–(9), respectively, versus NpNn. We note without details that the magnitude of VpairingNP is close to zero, and it is omitted here. One sees clearly that the magnitude of VSymNP is far larger than those of VSurfaceNP and VCoulombNP.

      The results of Eqs. (7)–(10) are very interesting, because all these contributions to the integrated neutron-proton interaction, which originated from the symmetry, surface, Coulomb and pairing energies in the mass formula of the liquid-drop model, are dominantly linear versus NpNn. This provides us with a simple explanation of the good correlation between VNP and NpNn, which was explored in the literature [810].

      In Fig. 2, we plot VsymNP, VsurfaceNP, and VCoulombNP for the case of the major shells of 82<N<126 and 50<Z<82. VpairNP is not plotted, because its value is always close to zero. From this figure, one sees that the contribution of VsymNP is dominant, while the two other contributions, i.e., those of VCoulombNP and VsurfaceNP, are far smaller. In fact, the relevance measurement of these terms can be clearly seen from Eqs. (7)–(10), where the ratios to NpNn for VsymNP, VsurfaceNP, VCoulombNP, and VpairNP, are approximately proportional to 1/A, 1/A4/3, 1/A4/3, and 1/A7/3, respectively.

    III.   CONTRIBUTIONS FROM WIGNER ENERGY AND SHELL EFFECT
    • In this section we discuss contributions from other two "residual" terms of binding energy in the liquid drop model: the Wigner energy term and the shell correction term in Eq. (3).

      The contribution to VNP from the Wigner energy is sizable only for the particle-particle or hole-hole case with valence protons and neutrons in the same major shells; otherwise, this contribution is very small and is negligible (mostly below 1 MeV) in comparison with the value of VNP, similar to the situation of VpairNP, and this is the case for the (50<Z<82, 82<N<126) shell. In this paper, for the sake of completeness, we investigate the particle-particle or hole-hole case with valence protons and neutrons in the same major shells.

      We assume that (Np+Nn)/(N+Z) is small and expand the contribution from the Wigner energy in terms of this ratio. For simplicity, we adopt the Wigner energy from Ref. [22]:

      Bw(Z,N)=W|NZ|Ad1AδN,Zπnp,

      (11)

      where W=42.7 MeV and d=28.7 MeV, according to Ref. [22]. We note that the results are very close to those obtained by assuming the Wigner energy of Refs. [19], without details. Here, πnp equals 1 for odd-odd nuclei and vanishes otherwise.

      Correspondingly, the contribution to VNP from the Wigner energy has two terms, which are denoted as VWNP and VdNP, respectively. The result of VdNP is simple and takes the following form. When N and Z are even and N=Z,

      VdNP=d4[1A0+21A+2];

      (12)

      and when N and Z are odd and N=Z,

      VdNP=d4[1A0+21A];

      (13)

      VdNP vanishes otherwise. From these results, one easily sees that VdNP is negligibly small in comparison with the value of VNP in all the regions that we discuss in this paper. For simplicity, one assumes VdNP0. The details of deriving VWNP are presented in Appendix A of this paper, and the final results are as follows. When the proton and neutron are in the same major shells,

      VWNP4WN+Z+2N0min(Np,Nn)

      (14)

      for the particle-particle case and

      VWNP4WN+Z+2N0min(Np,Nn)

      (15)

      for the hole-hole case [in Eq. (15), Np and Nn correspond to the numbers of holes]. According to the above two formulas, VWNP is proportional to Np (or Nn) when Np (or Nn) is smaller than Nn (or Np). Although the VWNP values in Eqs. (14)–(15) are not well linear-correlated with NpNn, they increase as Np and/or Nn increase. Furthermore, the values of VWNP are maximally approximately 10 MeV for the particle-particle and hole-hole cases when the proton and neutron are in the same major shell and thus are far smaller than VsymNP. In principle, VWNP breaks the linearity between VNP and NpNn in these two special cases, but this breaking is minor. We note again that the contribution of the Wigner energy to VNP is negligible when one investigates the (28<Z<50, 50<N<82) and (50<Z<82, 82<N<126) major shells, in which cases valence protons and neutrons are not in the same major shells.

      We finally come to the VshNP term, by adopting the calculated Bshell of Ref. [19]. The results for VshNP are plotted in terms of NpNn in Fig. 3. One sees that these VshNP values exhibit reasonable linearity with NpNn in most cases (with fluctuations), with the exception of the (50<Z<82, 82<N<126) major shells in which the magnitudes of VshNP increase when NpNn is below 100 and tend to be saturated when NpNn is larger than 100. However, all these VshNP values are far smaller than the corresponding VsymNP results. Additionally, the VshNP values of the hole-hole case are maximally approximately 12 MeV (positive), and those of the particle-hole case are maximally approximately 7 MeV (negative). We shall see soon that the sizable differences of VshNP between the hole-hole case and particle-hole (hole-particle) case are very important for explaining the subtle pattern of VNP versus NpNn, as observed in Refs. [10, 11].

      Figure 3.  (color online) The contribution to VNP from the shell correction part in the liquid drop model, for four major shells. Here, the shell correction energies are taken from the WS3 model.

    IV.   DISCUSSION
    • In this section, we discuss the implication of our derived formula for VNP.

      By summing all the above results of Eqs. (7)–(15), neglecting contributions from the Coulomb energy and pairing interaction [when one discusses the (28<Z<50, 50<N<82) and (50<Z<82, 82<N<126) major shells, the term VWNP is also negligible], the neutron-proton interactions are essentially given by

      VNPVsymNP+VshNP+VWNP.

      (16)

      By using Eq. (16), VsymNP of Eq. (7), the VshNP extracted by the shell correction results of Ref. [19], and VWNP of Eqs. (14) and (15), we obtain VNP and plot it versus NpNn in panels (a-d) of Fig. 1(labeled as "this work"). One sees good agreement with the results in panels (a-d).

      It is interesting and also one of the purposes of this paper to explain subtle details of the pattern exhibited in Fig. 1. This pattern is very striking and well-known for nuclei in the (28<Z<50,50<N<82) and (50<Z<82, 82<N<126) major shells, for which Eq. (16) is reduced to

      VNPVsymNP+VshNP,

      (17)

      assuming that both VCoulombNP0 and VWNP0. Because the ratio of VsymNP to NpNn is dominantly of 1/A-dependence according to Eq. (7), the neutron-proton interaction is strongest for the particle-particle case, for which the mass number is the smallest among the four cases, i.e., particle-particle, particle-hole, hole-particle, and hole-hole. One therefore expects the ordering of VNP as follows. The VNP of the particle-particle case is the largest, that of the hole-hole case is the smallest, and that of the particle-hole and hole-particle cases is in-between.

      Interestingly, the above simple pattern is actually "refined", albeit slightly, by the VshNP term. This refinement is striking in particular for the (28<Z<50, 50<N<82) and (50<Z<82, 82<N<126) major shells. As shown in Fig. 3 and discussed in Sec. III, the VshNP values are positive for both the particle-particle and hole-hole cases and are negative for both the hole-particle and particle-hole cases. Therefore, the neutron-proton interactions for the particle-particle case is further enhanced by VshNP and thus is the largest among the four cases, i.e., the particle-particle, hole-hole, particle-hole, and hole-particle cases. For the particle-hole case and the hole-hole case of the (50<Z<82, 82<N<126) major shells, although the VsymNP results of the hole-hole case are the smallest, they are "lifted" up by approximately 12 MeV maximally, while the VsymNP results of the particle-hole case are reduced by maximally approximately 7 MeV. This competition is the key to explain the order inversion of VNP for the particle-hole and hole-hole cases. It is the term VshNP that reduces VNP for the particle-hole case and boosts VNP for the hole-hole case, thus yielding the order inversion of VNP for these two cases. This is precisely the pattern reported in Refs. [10, 11].

    V.   SUMMARY
    • To summarize, in this paper, we study the patterns of neutron-proton interactions (denoted by VNP) in a few major shells of the nuclide chart: (28<Z<50, 28<N<50), (28<Z<50, 50<N<82), (50<Z<82, 50<N<82), and (50<Z<82, 82<N<126). We show that the dominant part in VNP originates from the symmetry energy, whose contribution is approximately proportional to NpNn, i.e., the product of the valence proton number and valence neutron number. We note without details that this pattern is robust; i.e., one obtains essentially the same pattern if one replaces results of Ref. [19] by using those of Refs. [20] and [21], i.e., the Duflo-Zuker model and the finite-range-liquid-drop model.

      Contributions to the VNP from other parts in the liquid-drop model, such as the volume energy, surface energy term, and Coulomb energy term, are either zero or close to zero. The contribution from the Wigner energy is either very close to zero (when valence protons and neutrons are not in the same major shells) or far smaller than that from the symmetry energy term. The VNP values of these origins are demonstrated to be the largest for the particle-particle case and the smallest for the hole-hole case. However, the contribution to the VNP from the shell correction is positive for particle-particle and hole-hole cases and is negative for particle-hole and hole-particle cases. Therefore one has always the strongest VNP of the particle-particle case for all major shells. The competition of VsymNP, which is the smallest for the hole-hole case and in-between for the particle-hole and hole-particle cases, with VshNP, which is positive for the hole-hole case and negative for the particle-hole and hole-particle cases, yields an order inversion of VNP for the hole-hole and particle-hole cases, as observed in previous papers [10, 11].

    APPENDIX A: DETAILED DERIVATION
    • In the Appendix, we present the details to derive Eqs. (8)–(10), (14), and (15). We exemplify the derivations of the four cases, i.e., the particle-particle, hole-hole, particle-hole, and hole-particle cases, by using the particle-particle case only, as it would be redundant and tedious to present all four cases. The formulas for the other three cases can be obtained in the same way, and with the same form. The particle-particle case corresponds to δp=δn=1 in Eq. (1). The contributions of the different components to VNP, including VsymNP, VsurfaceNP, VCoulombNP, VpairNP, and VWNP, include 16 terms, according to the definition of the empirical VNP in Eqs. (1)–(2). In Sec. II, we present the derivation of [VsymNP]V.

      We first come to the VsurfaceNP term, with the surface energy of the mass formula defined by asA23. From the definition of VNP in Eqs. (1)–(2), we have

      VsurfaceNP=14[as(Z+N)2/3as(Z+N+2)2/3as(Z+N+1)2/3as(Z+N+1)2/3as(Z0+N0)2/3as(Z0+N0+2)2/3as(Z0+N0+1)2/3as(Z0+N0+1)2/3+as(Z0+N)2/3+as(Z0+N+2)2/3+as(Z0+N+1)2/3+as(Z0+N+1)2/3+as(Z+N0)2/3+as(Z+N0+2)2/3+as(Z+N0+1)2/3+as(Z+N0+1)2/3].

      By using the convention A0=N0+N0, Z=Z0+Np, and N=N0+Nn, the above formula is rewritten as follows:

      VsurfaceNP=14asA2/30[(1+Np+NnA0)2/3(1+Np+Nn+2A0)2/32(1+Np+Nn+1A0)2/31(1+2A0)2/32(1+1A0)2/3+(1+NnA0)2/3+(1+Nn+2A0)2/3+2(1+Nn+1A0)2/3+(1+NpA0)2/3+(1+Np+2A0)2/3+2(1+Np+1A0)2/3].

      We expand the right-hand side of VsurfaceNP in terms of Np/A0 and Nn/A0 and obtain

      VsurfaceNP14as[29+49[1+1/(Z0+N0)]4/3+29[1+2/(Z0+N0)]4/3]NpNn(Z0+N0)4/329asNpNn(Z0+N0)4/3.

      This gives Eq. (8).

      We next come to the contribution of Coulomb energy to VNP. We use the Coulomb energy in the mass formula to be acZ2A13(10.76Z23). Here, the contribution from the first term is called the direct term, which is denoted as[VCoulombNP]d. As in VsurfaceNP, [VCoulombNP]d has also 16 terms and can be written as follows.

      [VCoulombNP]d=14acA5/30×[(Z0+NpA0)2(1+Np+NnA0)1/3(Z0+Np+1A0)2(1+Np+Nn+2A0)1/3(Z0+Np+1A0)2(1+Np+Nn+1A0)1/3(Z0+NpA0)2(1+Np+Nn+1A0)1/3(Z0A0)2(Z0+1A0)2(1+2A0)1/3(Z0+1A0)2(1+1A0)1/3(Z0A0)2(1+1A0)1/3+(Z0A0)2(1+NnA0)1/3+(Z0+1A0)2(1+Nn+2A00)1/3+(Z0+1A0)2(1+Nn+1A0)1/3+(Z0A0)2(1+Nn+1A0)1/3+(Z0+NpA0)2(1+NpA0)1/3+(Z0+Np+1A0)2(1+Np+2A0)1/3+(Z0+Np+1A0)2(1+Np+1A0)1/3+(Z0+NpA0)2(1+Np+1A0)1/3].

      We expand all these terms in terms of NpA0 and NnA0, yielding

      [VCoulombNP]d14ac(A0)5/3[2Z0A03(1+1A0)4/34(Z0A0)29(1+1A0)7/3+2(3+12Z0A0)(1+Z0A0)9(1+1A0)7/3+2(4+42Z0A0)(1+Z0A0)9(1+2A0)7/329(3Z0A0+2(Z0A0)2)]1(A0)2NpNnac[23Z0(Z0+N0)4/349Z20(Z0+N0)7/3]NpNn.

      This gives the first term of Eq. (9). The second term in Eq. (9) is obtained in the same way.

      In Eqs. (1)–(3), the definition of the pairing energy is

      Bpair(Z,N)=apairA13δnp.

      Here, δnp is defined as

      δnp={2|I|: {\it N} and {\it Z} even|I|: {\it N} and {\it Z} odd1|I|: {\it N} even, {\it Z} odd, and {\it N} > {\it Z} 1|I|: {\it N} odd, {\it Z} even, and {\it N} < {\it Z} 1: {\it N} even, {\it Z} odd, and {\it N} < {\it Z} 1: {\it N} odd, {\it Z} even, and {\it N} > {\it Z} ,

      with isospin asymmetry I=(NZ)/A. As an approximation, we assume that (N+Z+1)1/3 and (N+Z+1)1/3 are equal to (N+Z)1/3; NZN+Z+2 and NZ+1N+Z+1 are equal to (NZ)N+Z, and to exemplify the derivation of VpairNP with N>Z and both (Z, N) odd, we have

      VpairNPapair[(N+Z)1/3(4|NZ|N+Z)+(N0+Z0)1/3(4|N0Z0|N0+Z0)(N0+Z)1/3(4|N0Z|N0+Z)(N+Z0)1/3(4|NZ0|N+Z0)]apair[491(Z0+N0)7/3+79N0Z0(Z0+N0)103]NpNn,

      This gives Eq. (10) for the N>Z case. In all cases of Eq. (23), VpairNP is negligibly small in the VNP-NpNn plot.

      The Wigner energy is defined in Eq. (11). The contribution to the VNP from the second term is very simple and is given by Eqs. (12)–(13). The contribution from the first term, i.e., W|NZ|A, has 16 terms, which can be simplified by using the assumption that N+Z, N0+Z0, N0+Z, and N+Z0 plus 0 or 1 or 2 in the denominators equal (N+N0+Z+Z0)/2. We have

      VWNPW2(N+N0+Z+Z0)[2|NZ||NZ+1||NZ1|2|N0Z0||N0Z0+1||N0Z01|+2|NZ0|+|NZ0+1|+|NZ01|+2|N0Z|+|N0Z+1|+|N0Z1|].

      In most cases, NZ1, and under this assumption, one has

      VWNP2WN+N0+Z+Z0[|NZ||N0Z0|+|NZ0|+|N0Z|].

      Clearly, as expected, when valence protons and neutrons are not in the same major shells or when valence protons and neutrons are in the same major shells for the particle-hole and hole-particle cases, VWNP and VWNP equal zero in the above formula (in the realistic case, they are very close to zero). For the particle-particle case with valence protons and neutrons in the same major shells, one has

      VWNP4WN+Z+2N0(min{N,Z}N0);

      for the hole-hole case with valence protons and neutrons in the same major shells,

      VWNP4WN+Z+2N0(N0max{N,Z}).

      The above two formulas give Eqs. (14)–(15).

Reference (22)

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