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It is known that the half-life of elements decreases with increasing atomic number. As a result, the synthesis of superheavy elements is challenging. By contrast, nuclear research has foreseen the existence of a so-called “stability island” for certain superheavy elements of the nuclide chart, which accordingly ought to have half-lives starting from several minutes to several years. Achieving this stability island will produce super-heavy nuclei with a half-life long enough to conduct real experiments [1].
Superheavy nuclei are produced through a fusion action in heavy ion collisions with different methods. One of these methods involves the concept of dinuclear system (DNS) model, which works well to describe the fusion in reactions producing superheavy nuclei [2-7]. At energies around the Coulomb barrier for heavy ion collisions, after mutual capture of colliding nuclei, a moleculelike nuclear configuration (so-called nuclear molecule or DNS) is probably to form [5-7]. At this step, nucleons are exchanged between two nuclei as far as the DNS evolves to the equilibrium. Before compound nucleus (CN) formation, owing to Coulomb repulsion, the DNS may separate again (approximately
10−21 –10−20 sec.), which is called quasi-fission (QF) [8].A nuclear molecule or DNS consists of two touching nuclei that move within the internuclear distance with the transfer of nucleons. Consequently, this system consists of two main degrees of freedom: (1) the exchange of nucleons between the projectile and target nuclei, and (2) the relative motion between two nuclei, leading to fusion-fission and QF, respectively. QF and fusion-fission are severe obstacles to the formation of a superheavy nucleus. The principal difference between QF and fusion-fission is that a CN is not formed during the QF process [9-11].
Generally, heavy nuclei are produced in three stages: capture, fusion, and deexcitation. Studying each of these stages can help us understand and analyze the production of heavy nuclei.
In this study, we aimed to find an appropriate DNS for the formation of
296 119 superheavy compound nucleus. This nucleus was chosen because the highest known atomic number to date belongs to the Oganesson nucleus, which has 118 protons [12-14]. For this purpose, we considered four reactions for the production of296 119 superheavy element, including45 Sc +251 Cf,42 Ca +254 Es,39 K +257 Fm, and38 Ar +258 Md. These reactions were selected for the following reasons: (1) projectiles are stable nuclei; (2) targets are nuclei that have an alpha decay; (3) targets are actinides; and (4) three of the projectiles have a magic number (4220 Ca,3919 K, and3818 Ar), with two of them having a closed neutron shell (3919 K and3818 Ar), and one of them having a closed proton shell (4220 Ca). In other words, all types of nuclei (even-odd, odd-odd, and even-even nuclei) are used in reactions. Selective reactions can be discussed only from a theoretical point of view; many reactions considered cannot be used owing to lack of target material.It needs to be said that projectiles heavier than
48 Ca are commonly selected for the synthesis of superheavy nuclei with proton numbers greater than 118 [15]. This was the case in a number of previous studies [16-22] in which two reactions were suggested for production of the element with 119 protons, namely48 Ca +252 Es and50 Ti +249 Bk, which lead to the formation of 300119 and 299119 nuclei, respectively. However, in this study, we aimed to study the behavior of projectiles lighter than48 Ca for the synthesis of a superheavy nucleus with 119 protons.This paper reviews the driving potential in the framework of the two-center shell model (TCSM) and the folding potential in Section II. The results are presented in Section III in the form of capture, fusion, and evaporation residue cross sections, and survival probability calculations. Finally, the conclusions drawn from our calculations are provided in Section IV.
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The potential energy for heavy nuclear configuration plays a crucial role for the understanding of the evolution of the collision of nuclei. Thus, it is better to start with the driving potential. The potential energy surface that controls the evolution of a nuclear system in a multi-dimensional space is commonly called “driving potential” [23]. In other words, the driving potential includes a value of nucleus-nucleus potential corresponding to the minimum of its potential well.
The potential energy depends on three parameters: (1) the mass asymmetry (
η ), which is defined as the ratio of the subtraction of the mass of two colliding nuclei to their sum, (2) the distance between mass centers of the colliding nuclei (r), and (3) the neck parameterε [24-26], which is determined as the ratio of the height of the smoothed potential to the original one [27]. For fusion reaction, a realistic value of the neck parameter isε = 1.The potential energy of the separated nuclei is defined as the interaction energy of the colliding nuclei, which might be calculated using the double-folding method, proximity potential, or Bass model (for spherical nuclei). By crossing the fusion barrier, the further evolution of the system may be an adiabatic or diabatic process (owing to the relative movement speed of the two nuclei) [23, 24]. Using the code in Ref. [24], one can calculate the multi-dimensional diabatic (in the folding model framework) and adiabatic (in the TCSM framework) driving potentials. As seen in Fig. 1, diabatic and adiabatic processes must have the same potential before the two nuclei touch, but after touching, these processes exhibit quite different behavior. In the diabatic process, the two nuclei approach each other rapidly, and after contact, they try to penetrate each other, and the potential energy increases rapidly. In contrast, in the adiabatic process, the nuclei slowly approach each other, and the DNS has sufficient opportunity to change its configuration to hold the nuclear density and to keep the potential energy from exceeding a certain limit. In this study, we used the adiabatic process for potential driving after touching. Moreover, we considered the axially symmetric configurations.
Figure 1. (color online) Potential energy as elongation function for the nuclear system formed by (a)
45 Sc +251 Cf, (b)42 Ca +254 Es, (c)39 K +257 Fm, and (d)38 Ar +258 Md in the framework of TCSM compared with the folding potential.In Fig. 1, the TCSM is used in the form of an adiabatic process to consider the shell effect, and the folding potential is used in the form of a diabatic process to consider the effects of deformation and orientation. The underlying theory is detailed in Secs. IIB and IIC.
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The TCSM Hamiltonian in cylindrical coordinates is defined as the sum of potential and kinetic energies, comprising three terms: a two-center oscillator, spin-orbit, and
l2 -terms [28-30]:ˆHTCSM=−ℏ22m0∇2+V(z,ρ)+VLS(r,p,s)+VL2(r,p),
(1) where
z1 andz2 denote the places of the centers, and the momentum independent term of the potential is given byV(z,ρ)=12m0{(ω2z1z′2+ω2ρ1ρ2),z<z1[ω2z1z′2(1+c1z′+d1z′2)+ω2ρ1ρ2(1+g1z′2)],z1<z<0[ω2z2z′2(1+c2z′+d2z′2)+ω2ρ2ρ2(1+g2z′2)],0<z<z2(ω2z1z′2+ω2ρ1ρ2),z>z2
(2) where
z′={z−z1,z<0z−z2,z>0
(3) the potential of the spin-orbit interaction is
VLS(r,p,s)={{−ℏκ1m0ω01,(∇V×p)⋅s}, z<0{−ℏκ2m0ω02,(∇V×p)⋅s}, z>0
(4) and the
VL2 potential isVL2(r,p)={−12{κ1μ1ℏω01,l2}+κ1μ1ℏω01N1(N1+3)2δif, z<0−12{κ2μ2ℏω02,l2}+κ2μ2ℏω02N2(N2+3)2δif, z>0
(5) In the above formula,
δif is a Kronecker symbol, and{x,y}≡xy+yx denotes the anticommutator of two quantities;ωρi andωzi are the oscillator frequencies inρ and z directions, respectively, and arezi -dependent. Moreover,κi is the spin-orbit interaction constant, andμi is the tunable parameter of the Nilsson model, which depends on the two-center distance. Finally,Ni=nρi+nzi(zi) denotes the principal quantum number of the two-center oscillator, which is azi -dependent quantity, wherenzi is the solution of a transcendental equation andnρi is a nonnegative integer;ℏω0i=41/˜A1/3i is the energy level spacing of the spherical oscillator, where˜Ai is the mass number of the nuclear fragment [28-30].The potential mentioned in Eqs. (1-5) refers to a single-particle potential. We used the TCSM for the calculation of the adiabatic potential energy of the nucleus-nucleus interaction that can be found in [24].
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The double-folding model is one of the most common methods to determine the internuclear potential for heavy ion interaction that includes the sum of the effective interaction of the nucleon-nucleon. The interaction energy of two nuclei in the folding model is calculated as [23, 24, 31]
V12(r;δ1,Ω1,δ2,Ω2)=∫ V1ρ1(r1)∫ V2ρ2(r2)vNN(r12)d3r1d3r2,
(6) in this formula,
r12=r+r2−r1 , andvNN(r12) denotes the effective interaction of the nucleon-nucleon, which includes two parts: nuclear and Coulomb. Moreover,ρ1(r1) andρ2(r2) are the distributions of the nuclear matter density within the colliding nuclei, which is often calculated asρ(r)=ρ0[1+exp(r−R(Ωr)a)]−1,
(7) Ωr are the spherical coordinates of r, andR(Ωr) denotes the distance to the nuclear surface. The amount ofρ0 is specified by the condition∫ρid3r=A . A more detailed description of the folding potential can be found in [31].Figure 2 shows the driving potentials as a function of the
η parameter in the framework of TCSM for the DNS leading to296119 . Note in this figure that there are two minima in the driving potential atη=0.07 andη=0.4 for the reactions atRB (derived from Ref. [24]); the minimum potential energy for these minima are listed in Table 1. This figure also shows the value of the internal fusion barrierB∗fus . The important property of the DNS evolution to the CN is the existence of a fusion barrierB∗fus in the mass asymmetry coordinate. The value of the internal fusion barrier determines a hindrance for complete fusion that the DNS must overcome to form a CN [4].Figure 2. (color online) Driving potential as a one variable function (
η ) for the DNS leading to the296119 CN formed by (a)45 Sc +251 Cf, (b)42 Ca +254 Es, (c)39 K +257 Fm, and (d)38 Ar +258 Md in the framework of TCSM. The red line indicates the entrance channel. The value of the internal fusion barrier for each reaction is also shown.Reaction RB/fm Mass asymmetry ( η )Minimum potential energy/MeV First (η=0.07) Second (η=0.4) 45 Sc+251 Cf 12.716 0.696 179.3 179.7 42 Ca+254 Es 12.675 0.716 169.9 170.2 39 K+257 Fm 12.630 0.736 157.3 157.6 38 Ar+258 Md 12.622 0.743 153.9 154.3 Table 1. Minimum value of the driving potential (in the TCSM) as a function of
η in the targeted reactions.By using the code in Ref. [24], we show in Fig. 3 the driving potential as a function of the proton number of the DNS leading to an identical CN with A = 296 and Z = 119 (in contact point). This figure is equivalent to Fig. 2. It is clear from Figs. 2 and 3 that the amount of internal fusion barrier in the
38 Ar +258 Md reaction is smaller than for other studied reactions.Figure 3. (color online) Driving potential calculated for the DNS leading to an identical CN with A = 296 and Z = 119 as a function of the proton number of the DNS formed by (a)
45 Sc +251 Cf, (b)42 Ca +254 Es, (c)39 K +257 Fm, and (d)38 Ar +258 Md reactions. The red arrow indicates the initial proton number of the projectile for the targeted reaction.The landscape of the potential energy surface specifies the competition between complete fusion and QF during the evolution of the DNS [32]. For this purpose, the dependence of the potential energy on the polar orientation for each reaction was studied. In Fig. 4, this dependence on the orientation with the parameter R can be observed. This figure shows that the parameters of the fusion barriers strongly depend on the orientation of the nuclei during fusion [23, 25, 26]. According to this figure, the minimum and maximum energies occur at
0∘ (nose-to-nose collision) and±90∘ (side-by-side collision), respectively. Furthermore, as expected, the maximum energy occurs around the point contact. The minimum energy at the point contact is at0∘ for the considered reactions; the corresponding values are listed in Table 2.Figure 4. (color online) Dependence of the potential energy on mutual orientation in the reaction plane and R (distance between mass centers of colliding nuclei) in (a)
45 Sc +251 Cf, (b)42 Ca +254 Es, (c)39 K +257 Fm, and (d)38 Ar +258 Md reactions. The mutual orientation is such that0∘ and±90∘ angles show nose-to-nose and side-by-side collisions, respectively.Reaction Minimum energy ( Rcontact )45 Sc+251 Cf 183.48 MeV (12.03 ± 0.06 fm)42 Ca+254 Es 181.27 MeV (12.05 ± 0.06 fm)39 K+257 Fm 178.79 MeV (11.95 ± 0.06 fm)38 Ar+258 Md 168.34 MeV (11.90 ± 0.06 fm)Table 2. Minimum potential energy obtained from the reactions at
0 degree orientation of the colliding nuclei. The corresponding point contact is given inside the parentheses. -
In the fusion of superheavy ions, the CN formation probability after touching of two nuclei is less than unity due to the QF processes. In such systems, the cross section of fusion corresponds to the so-called “capture cross section”, which is defined as the QF cross section (without CN formation) plus the fusion cross section (CN formation). The total capture cross section is [3, 23, 25, 26]
σcap(E,l)=πλ−−2∞∑l=0(2l+1)Tl(E),
(8) where
λ−− represents the reduced De-Broglie wavelength, andσcap(E) describes the transition of two nuclei on the Coulomb barrier with the primary dinuclear system formation;Tl(E) denotes the probability that the angular momentum l of the relative motion converts into the DNS angular momentum in the center-of-mass energy framework. Moreover, as mentioned before, the kinetic energy is converted into excitation energy as well [33, 34]. The probability of these changes is defined by the Hill-Wheeler equation [35]:THWl(B,E)=(1+exp(2πℏωB(l)[B+ℏ22μR2B(l)l(l+1)−E]))−1,
(9) where
ℏωB=√ℏ2/μ|∂2V/∂r2|B represents the potential barrier width, B denotes the barrier height, andRB(l) represents the position of the effective barrier that contains a centrifugal part. The penetration probability for spherical nuclei is the average over B [24-26]:Tl(E)=∫F(B)THWl[B(β);E]dB,
(10) where
F(B) can be approximated by a symmetric Gaussian [24-26]:F(B)=N.exp(−[B−B0ΔB]2),
(11) where
B0=(B1+B2)/2 andΔB=(B2−B1)/2 . The quantityB1 depends on dynamic deformation andB2 is the Coulomb barrier of spherical nuclei.For our studied reactions, which consist of a spherical projectile and statically deformed target, the penetration probability must be averaged on the deformation-dependent barrier height and the colliding nuclei orientations. The Coulomb barrier height depends on the dynamic deformation of the projectile. Therefore, the probability of penetration is as follows [24]:
Tl(E)=∫π0sinθ22dθ2∫F(B′)THWl[B(θ,β);E]dB′,
(12) and considering (
θ ) as a target orientation and (β ) as a projectile deformation, the relationship between B andB′ to parameterize the barrier B for the arbitrary value of the (θ ) and (β ) is as follows [24]:B(θ,β)=B′+[B(θ,0),B(0,0)], B′=B(0,β).
(13) The effective nucleus-nucleus potential that can be seen inside the brackets in Eq. (9) is approximated around the Coulomb barrier by the potential of the inverted harmonic oscillator with frequency
ω(l) , and the maximum amount of angular momentum (lmax ) is determined by either the kinematical angular momentum aslkin={2μ[Ec.m.−V(Rb, Zi, Ai, β1=0, β2=0, l)]}1/2Rb/ℏ or by the critical angular momentum aslmax = minimum{ lkin ,lcr } [36]. The value of the critical angular momentum used for the reactions analyzed in this study is specified in Table 3.reactions critical angular momentum 45 Sc+251 Cf 121 42 Ca+254 Es 119 39 K+257 Fm 116 38 Ar+258 Md 116 Table 3. Amount of critical angular momentum used in the studied reactions.
Fig. 5 shows the calculated cross section of the fusion and capture. The difference between these cross sections is due to the absence of the CN in the QF process [9, 10].
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The cross section of the CN (fusion) is calculated as [16]
σfus(E,l)=πℏ22μE∞∑l=0(2l+1)Tl(E)PCN,
(14) PCN is the fusion probability that leads to the compound nucleus formation. The difference betweenσfus andσcap is encoded in aPCN coefficient, which is generally considered in the computation such that, for a CN with a probability of 100%,PCN=1 . Thus, in a heavy system, the capture process within the Coulomb barrier or DNS formation is not the enough condition for fusion but is the necessary condition for fusion [33, 34]. A simple parameterization ofPCN was proposed in [37, 38]:PCN(E,l)=exp(−c(xeff−xthr))1+exp(E∗B−E∗int(l)Δ),
(15) where the excitation energy of CN (at the Bass barrier) is denoted by
E∗B . Moreover,E∗int(l)=E−Erot(l)+Q is the inner excitation energy, which describes the damping of the shell correction to the CN fission barrier,Δ is the tunable parameter for approximately 4 MeV, Q is the fusion Q-value, andErot(l)=ℏ22Ig.s.l(l+1) is the rotational energy [16, 23, 25]. Furthermore, c,xeff , andxthr can be found in [37, 38].According to Table 4, the maximum values for
σfus andσcap in the reaction38 Ar +258 Md are greater than those for the other reactions studied; moreover, this reaction requires lower energy. It can be said that, as the mass asymmetry parameter (η ) increases, the maximum values for the fusion and capture cross sections increase as well (see Tables 2 and 4 ).Reaction Maximum capture cross section ( Ecm )Maximum fusion cross section ( Ecm )45 Sc+251 Cf 855.234 mb (275 ± 2.5 MeV)0.859 mb (265 ± 2.5 MeV)42 Ca+254 Es 861.806 mb (255 ± 2.5 MeV)5.921 mb (260 ± 2.5 MeV)39 K+257 Fm 954.991 mb (255 ± 2.5 MeV)39.891 mb (255 ± 2.5 MeV)38 Ar+258 Md 1005.70 mb (245 ± 2.5 MeV)200.349 mb (245 ± 2.5 MeV)Table 4. Maximum values for
σcap andσfus in this study. -
The formation cross section of the evaporation residue for heavy nuclei collisions is given as follows [39]
σEvR(Ec.m.)=Jmax∑J=0σcap(Ec.m.,J)PCN(Ec.m.,J)Wsur(Ec.m.,J),
(16) where the three coefficients are the cross section of capture, complete fusion probability, and survival probability. The cross section of capture,
σcap , describes the DNS formation in the first step of collision when kinetic energy (due to the relative movement) is converted into other energies (excitation energy and potential energy). Once formed, the DNS evolves within the coordinate of the mass asymmetryη . The mass distribution center moves in the direction of greater symmetric fragmentations. If part of the mass distribution passes through the internal fusion barrierB∗fus of the driving potentialU(η) , it gives rise to a probability of complete fusionPCN . Moreover, during this evolution, the DNS can decay with QF. Hence, the charge and mass distributions of the QF and the probability of the fusionPCN should work simultaneously [39].The excitation energy of the formed compound nucleus is approximately
E∗ = 30-40 MeV (orEcm = 180-190 MeV), and the transition of the excited compound nucleus to the ground state results in the emission of 3 or 4 neutrons from its surface [40]. Figure 6 shows the calculated evaporation residue cross sections for the 3n and 4n channels in the combinations studied. It is clear that the values ofσEvR in the38 Ar +258 Md reaction for both channels are greater than those for other reactions. This is a good sign that distinguishes this reaction from the reactions mentioned for the production of the296 119 superheavy element. -
For an excited CN, the probability to achieve a ground state with the emission of a neutron (or neutrons) is defined as “survival probability” and denoted by
Wsur [39]. This probability computes the contest among particle evaporation in thexn,yp,zα channel, the excited CN fission, and other particle evaporation channels [41, 42]. Therefore, the total survival cross section is the sum of the survival probability over all channels:σsurv(E,l)=πλ−−2∞∑l=0(2l+1)Tl(E)PCN(E,l)∑xn,yp,zαWxn,yp,zαsurv(E,l),
(17) Using the following equation, the survival probability for the 1n-evaporation channel is obtained:
W1nsur(Ec.m.,J=0)=Γn(E∗CN)Γf(E∗CN)=4A2/3(E∗CN−Bn)k(2[a(E∗CN−Bf)]1/2−1)exp[2a1/2(√E∗CN−Bn−√E∗CN−Bf)],
(18) where k = 9.8 MeV and
E∗CN=Ec.m.+Q . Moreover,a=(A1+A2)/12 is the ratio for the level density, whose value in the evaporation channels is equal to one;Bf is the fission barrier for the heaviest nuclei, whose amount is proportional to the CN excitation energy (Ec.m. ) asBf=Bf(E∗CN=0)exp[−E∗CN/Ed] , withEd=0.4A4/3/a [3, 33, 34].Previous studies showed that the probability of the survival is strongly proportional to the properties of the nuclear structure for the superheavy nuclei like deformation and level density [31]. We applied these properties in our calculations.
The results of calculation for
Wsur andσEvR in the 1-4n channels (in the range of 180-200 MeV) for the3818 Ar +258101 Md reaction by using codes in Ref. [24] are shown in Fig. 7. According to this figure, the maximum value forσEvR at the 3n-channel and 4n-channel are 0.18 (pb) and 0.05 (pb), respectively, which is in good agreement with previously reported results [16-22] for the production of an element with 119 protons. The variety of results may be related to the various methods, potentials, energy range, and neutron numbers of the element. -
We used several codes available in Ref. [24] to study the formation of
296 119 superheavy compound nucleus at energies near the Coulomb barrier. Our calculations and studies lead to the following conclusions.For the reactions with a larger mass asymmetry parameter, the minimum potential value in the contact point is further reduced. Thus,
4220 Ca,3919 K, and3818 Ar, which are spherical and magic nuclei, have a greater amount than4521 Sc in the capture (even fusion) cross section and survival probability. For3919 K and3818 Ar, which have closed neutron shells, the survival probability for CN is greater than other studied reactions without closed neutron shells; however, for4220 Ca, which has closed proton shells, the CN survival probability is less than those of nuclei with closed neutron shells. Moreover, as the mass asymmetry parameter (η ) increases, the maximum values for the capture and fusion cross sections increase as well.Although the maximum values for the capture and fusion cross sections are higher in the reaction
38 Ar +258 Md, it is not accurate to conclude that this reaction is the optimal one among the mentioned four combinations just based on the fusion cross sections. This is because the excitation energy of the compound nucleus could be much higher, thereby suppressing the survival probability. However, this reaction is a suitable choice for the formation of an element with 119 protons among our studied reactions, because the calculated evaporation residue cross section in the38 Ar +258 Md reaction is larger than those of other reactions; moreover, this reaction has a smaller fusion barrier.
Study of the dinuclear system for 296119 superheavy compound nucleus in fusion reactions
- Received Date: 2020-10-30
- Available Online: 2021-04-15
Abstract: This investigation aims to find an appropriate dinuclear system for the formation of